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The Nature of the Hydrogen Bond

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Gastone Gilli 作者
Oxford University Press, USA
译者
2009-8-25 出版日期
304 页数
USD 130.00 价格
Hardcover
丛书系列
9780199558964 图书编码

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The Nature of the Hydrogen Bond 在线电子书 epub 下载 mobi 下载 pdf 下载 txt 下载 2025

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The Nature of the Hydrogen Bond 在线电子书 pdf 下载 txt下载 epub 下载 mobi 下载 2025



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Hydrogen bond (H-bond) effects are known: it makes sea water liquid, joins cellulose microfibrils in trees, shapes DNA into genes and polypeptide chains into wool, hair, muscles or enzymes. Its true nature is less known and we may still wonder why O-H...O bond energies range from less than 1 to more than 30 kcal/mol without apparent reason. This H-bond puzzle is re-examined here from its very beginning and presented as an inclusive compilation of experimental H-bond energies and geometries. New concepts emerge from this analysis: new classes of systematically strong H-bonds (CAHBs and RAHBs: charge- and resonance-assisted H-bonds); full H-bond classification in six classes (the six chemical leitmotifs); and assessment of the covalent nature of strong H-bonds. This leads to three distinct but inter-consistent models able to rationalize the H-bond and predict its strength, based on classical VB theory, matching of donor-acceptor acid-base parameters (PA or pKa), or shape of the H-bond proton-transfer pathway. Applications survey a number of systems where strong H-bonds play an important functional role, namely drug-receptor binding, enzymatic catalysis, ion-transport through cell membranes, crystal design and molecular mechanisms of functional materials.

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